Issue

Vol. 18 (2026)

Interfacial Engineering Enables Flexible Composite Film Achieving Ultrahigh Thermal Conductivity and Wave Transparency

https://doi.org/10.1007/s40820-026-02297-3
Kaiyuan Li
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Linhong Li
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Guichen Song
Gansu Engineering Research Center of Eco‑Environment Intelligent Networking, College of Electrical Engineering, Northwest Minzu University, Lanzhou 730000, People’s Republic of China
Yue Qin
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Hanxi Chen
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Zujian Zhao
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Boren Yang
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Yiwei Zhou
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Yandong Wang
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Rongjie Yang
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Maohua Li
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Fei Chen
School of Integrated Circuits, Engineering Research Center for Functional Ceramics MOE, Huazhong University of Science and Technology, Wuhan 430074, People’s Republic of China
Tao Cai
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Cheng‑Te Lin
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Kazuhito Nishimura
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Nan Jiang
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China
Jinhong Yu
State Key Laboratory of Advanced Marine Materials, Zhejiang Key Laboratory of Extreme‑environmental Material Surfaces and Interfaces, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, People’s Republic of China

Corresponding Author: Jinhong Yu

yujinhong@nimte.ac.cn

Nano-Micro Letters, Vol. 18 (2026), Article Number: 439

Abstract

With the trend toward high-power radio-frequency (RF) electronic devices, flexible thermally conductive composite films are regarded as a key engineering interfacial material to address the critical problem of signal transmission and heat dissipation. However, achieving simultaneous optimization of high thermal conductivity and low loss in the same material remains a significant challenge, particularly in films with high filler loading. Here, a bottom-up regulatory strategy is proposed to address this challenge. Through the synergistic optimization of interface modification design and spatial orientation arrangement of hexagonal boron nitride (BN), the fabricated composite film achieves an exceptional in-plane thermal conductivity of 78.50 W m⁻1 K⁻1, significantly surpassing that of the film with BN. This remarkable enhancement is primarily attributed to the altered surface properties of the aminated BN (BN-NH2). The introduction of amine groups enhances the compatibility with the polymer matrix through electrostatic interactions to facilitate more efficient interfacial thermal transport. Furthermore, the highly oriented spatial arrangement of BN in the film not only preserves the electromagnetic wave transparency (99.94%), but also enhances its breakdown strength. This study underscores the critical role of molecular-level filler modification combined with micro-nanostructural engineering in synergistically strengthening the filler-matrix interface and boosting film thermal transport.


Highlights:
1 Through synergistic modulation of interface modification and spatial orientation, the scalable fabrication of BN-based thermal management films has been achieved.
2 The resulting films exhibit exceptional thermal conductivity reaching 78.50 W m−1 K−1 and electromagnetic wave transmittance over 99.9%, positioning this work at the forefront of the field.
3 This film demonstrates considerable potential for application in interfacial signal integrity and thermal management in radio-frequency electronic devices.

Keywords

Hexagonal boron nitride Surface functionalization Thermal conductivity Wave transparency
Li, Kaiyuan, Linhong Li, Guichen Song, Yue Qin, Hanxi Chen, Zujian Zhao, Boren Yang, Yiwei Zhou, Yandong Wang, Rongjie Yang, Maohua Li, Fei Chen, Tao Cai, Cheng‑Te Lin, Kazuhito Nishimura, Nan Jiang, and Jinhong Yu. 2026. “Interfacial Engineering Enables Flexible Composite Film Achieving Ultrahigh Thermal Conductivity and Wave Transparency”. Nano-Micro Letters 18 (July):439. https://doi.org/10.1007/s40820-026-02297-3.
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